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梅梁湾、大太湖夏季和冬季CDOM特征及可能来源分析

张运林, 秦伯强

张运林, 秦伯强. 梅梁湾、大太湖夏季和冬季CDOM特征及可能来源分析[J]. 水科学进展, 2007, 18(3): 415-423.
引用本文: 张运林, 秦伯强. 梅梁湾、大太湖夏季和冬季CDOM特征及可能来源分析[J]. 水科学进展, 2007, 18(3): 415-423.
ZHANG Yun-lin, QIN Bo-qiang. Feature of CDOM and its possible source in Meiliang bay and Da Taihu lake in Taihu lake in summer and winter[J]. Advances in Water Science, 2007, 18(3): 415-423.
Citation: ZHANG Yun-lin, QIN Bo-qiang. Feature of CDOM and its possible source in Meiliang bay and Da Taihu lake in Taihu lake in summer and winter[J]. Advances in Water Science, 2007, 18(3): 415-423.

梅梁湾、大太湖夏季和冬季CDOM特征及可能来源分析

基金项目: 江苏省自然科学基金资助项目(BK2006580);中国科学院优秀博士学位论文、院长奖获得者科研启动专项资金资助项目;中国科学院南京地理与湖泊研究所所长科研专项基金资助项目
详细信息
    作者简介:

    张运林(1976- ),男,湖南邵阳人,助理研究员,主要从事水光学、水生态学和水质遥感研究.E-mail:ylzhang@niglas.ac.cn

  • 中图分类号: X524

Feature of CDOM and its possible source in Meiliang bay and Da Taihu lake in Taihu lake in summer and winter

Funds: The study is financially supported by the Natural Science Foundation of Jiangsu Province(BK2006580),and by Scientific Research SpecialFoundation for Excellent Doctoral Dissertation and Decanal Schalarship of the CAS and the Scientific Resarch Special Foundation from NanjingInstitute of Geography and Limnology,Chinese Acdemy of Sciences.
  • 摘要: 基于2004年夏季水华暴发期和冬季在梅梁湾及大太湖各2次采样,分析了夏季、冬季CDOM的特征及其可能的来源,发现夏季CDOM吸收系数、叶绿素a浓度均明显高于冬季,DOC浓度、CDOM吸收系数a(355)的变化范围分别为5.17~12.42 mg/L、2.57~6.77 m-1,最大值均出现在冬季(12月15日)的直湖港入湖口.CDOM吸收系数与DOC浓度、定标后的荧光值一般都存在显著正相关,但夏季由于受浮游植物降解的影响,与DOC浓度和荧光的相关性明显低于冬季.表征CDOM组成和来源的参数比吸收系数、M值、S值存在显著的季节差异,夏季吸收系数a*(355)值明显要大于冬季,而S值、M值则要小于冬季.夏季水华暴发时CDOM吸收系数与叶绿素a浓度空间分布较为一致,吸收系数与叶绿素a浓度存在正相关,浮游植物降解产物可能是水体中CDOM的重要来源;相反,冬季CDOM吸收系数呈现从梁溪河入湖口、湾内往湾口递减的趋势,其来源可能主要以陆源为主,受入湖河流的影响较大.
    Abstract: The feature Chromophoric dissolved organic matter(CDOM) and its source in Meiliang bay and Da Taihu lake in Taihu Lake are analysed based on every 2 time's samplings in summer with algal bloom and winter.CDOM absorption coefficients and chlorophyll a concentration are significant higher in summer than winter.The DOC concentration and the CDOM absorption coefficients a(355) are in the range of 5.17-12.42 mg/L,2.57-6.77 m-1,respectively,with the maxima at the mouth of Zhihu river on Dec.15.Significant positive correlations are generally found within a(355),DOC concentration and normalized fluorescence Fn(355).The determination coefficients between a(355),DOC concentrations and Fn(355) are significantly lower in summer than winter due to the phytoplankton degradation.As the parameters representing the CDOM composition and the source,the DOC-specific absorption coefficients a*(355) are remarkably larger in summer than winter.However,M and S values are smaller in summer than winter with the seasonal variations.The spatial distribution of the CDOM absorption coefficients is similar to that of chlorophyll-a concentration in summer with algal bloom.A significant and positive correlation is found between a(355) and chlorophyll-a concentration,which shows that phytoplankton degradation is one of the potentially important sources of CDOM.By contrast,no significant correlation is found between a(355) and chlorophyll a concentration in winter.The CDOM absorption coefficient generally decreases from the mouth of river to the inlet and outlet of Meiliang bay,which shows that river terrestrial input is the potentially main source of CDOM.
  • [1] Williamson C E,Stemberger R S,Morris D P.Ultraviolet radiation in North American lakes:Attenuation estimates from DOC measurements and implications for plankton communities[J].Limnol Oceanogr,1996,41(5):1 024-1 034.
    [2] Laurion I,Ventura M,Catalan J,et al.Attenuation of ultraviolet radiation in mountain lakes:Factors controlling the among and within-lake variability[J].Limnol Oceanogr,2000,45:1 274-1 288.
    [3] 张运林,吴生才,秦伯强,等.太湖梅梁湾有色可溶性有机物对光的吸收[J].中国环境科学,2004,24(4):405-409.
    [4] Carder K L,Hawes S K,Baker K A,et al.Reflectance model for quantifying chlorophyll a in the presence of productivity degradation products[J].J Geophys Res,1991,96:20 599-20 611.
    [5] Doxaran D,Froidefond J M,Lavender S,et al.Spectral signature of highly turbid waters Application with SPOT data to quantify suspended particulate matter concentrations[J].Remote Sens Environ,2002,81:149-161.
    [6] Gao H,Zeep R G.Factors influencing photoreactions of dissolved organic matter in a coastal river of the southeastern United States[J].Environ Sci Technol,1998,32:2 940-2 946.
    [7] Kieber D J.Photochemical production of biological substrates[A].In de Mora S,Demers S,Vernet M eds,"The effect of UV radiation in the marine environment"[C].Cambridge:Cambridge University Press,2000.130-148.
    [8] 吴永森,张士魁,张绪琴,等.海水黄色物质光吸收特性实验研究[J].海洋与湖沼,2002,33(4):402-406.
    [9] 陈楚群,潘志林,施平.海水光谱模拟及其在黄色物质遥感反演中的应用[J].热带海洋学报,2003,22(5):33-39.
    [10] Callahan J,Dai M H,Chen R F,et al.Distribution of dissolved organic matter in the Pearl River Estuary,China[J].Mar Chem,2004,89:211-224.
    [11] 张运林,秦伯强,马荣华,等.太湖典型草、藻型湖区有色可溶性有机物的吸收及荧光特性[J].环境科学,2005,26(2):142-147.
    [12] Bricaud A,Morel A,Prieur L.Absorption by dissolved organic matter of the sea(yellow substance) in the UV and visible domain[J].Limnol Oceanogr,1981,26:43-53.
    [13] Green S,Blough N.Optical absorption and fluorescence properties of chomophoric dissolved organic matter in natural waters[J].Limnol Oceanogr,1994,39(8):1 903-1 916.
    [14] 陈宇炜,高锡云.浮游植物叶绿素a含量测定方法的比较测定[J].湖泊科学,2000,12(2):185-188.
    [15] Hoge F E,Vodacek A,Blough N V.Inherent optical properties of the ocean:retrieval of the absorption coefficient of chromophoric dissolved organic matter from fluorescence measurements[J].Limnol Oceanogr,1993,38:1 394-1 402.
    [16] De Haan H.Solar UV-light penetration and photodegradation of humic substances in peaty lake water[J].Limnol Oceanogr,1993,38:1 072-1 076.
    [17] Vodacek A,Hoge F E,Swift R N,et al.The use of in situ and airborne fluorescence measurements to determine UV absorption coefficients and DOC concentrations in surface waters[J].Limnol Oceanogr,1995,40:411-415.
    [18] Ferrari G M,Dowell M D,Grossi S,et al.Relationship between the optical properties of chromophoric dissolved organic matter and total concentration of dissolved organic carbon in the southern Baltic Sea region[J].Mar Chem,1996,55:299-316.
    [19] Del Vecchio R,Blough N V.Spatial and seasonal distribution of chromophoric dissolved organic matter and dissolved organic carbon in the Middle Atlantic Bight[J].Mar Chem,2004,89:169-187.
    [20] Nelson N B,Siegel,D A,Michaels A F.Seasonal dynamics of colored dissolved organic material in the Sargasso Sea[J].Deep-Sea Res Pt I,1998,45:931-957.
    [21] Chen Z Q,Li Y,Pan J M.Distributions of colored dissolved organic matter and dissolved organic carbon in the Pearl River Estuary,China[J].Cont Shelf Res,2004,24:1 845-1 856.
    [22] Rochelle-Newall E J,Fisher T R.Chromophoric dissolved organic matter and dissolved organic carbon in Chesapeake Bay[J].Mar Chem,2002,77:23-41.
    [23] Vodacek A,Blough N V,Degrandpre M D,et al.Seasonal variation of CDOM and DOC in the Middle Atlantic Bight:terrestrial inputs and photooxidation[J].Limnol Oceanogr,1997,42:674-686.
    [24] Del Castillo C E,Coble P G.Seasonal variability of the colored dissolved organic matter during the 1994~1995 NE and SW Monsoons in the Arabian Sea[J].Deep-Sea Research Ⅱ,2000,47:1 563-1 579.
    [25] Rochelle-Newall E J,Delille B,Frankignoulle M,et al.Chromophoric dissolved organic matter in experimental mesocosms maintained under different pCO2 levels[J].Mar Ecol Prog Ser,2004,272:25-31.
    [26] Kowalczuk P,Stedmon C A,Markager S.Modeling absorption by CDOM in the Baltic Sea from season,salinity and chlorophyll[J].Mar Chem,2006,101:1-11.
    [27] 李素菊.利用分析方法建立湖泊水质参数反演算法研究——以安徽巢湖为例[D].北京:北京大学,2003.
    [28] Kowalczuk P.Seasonal variability of yellow substance absorption in the surface layer of the Baltic Sea[J].J Geophys Res,1999,104:30 047-30 058.
    [29] Kahru M,Mitchell B G.Seasonal and nonseasonal variability of satellite-derived chlorophyll and dissolved organic matter concentration in the California Current[J].J Geophys Res,2001,106:2 517-2 529.
    [30] Sasaki H,Miyamura T,Saitoh S,et al.Seasonal variation of absorption by particles and colored dissolved organic matter(CDOM) in Funka Bay,southwestern Hokkaido,Japan[J].Estuar Coast Shelf S,2005,64:447-458.
    [31] Etheridge S M,Roesler C S.Temporal variations in phytoplankton,particulates,and colored dissolved organic material based on optical properties during a Long Island brown tide compared to an adjacent embayment[J].Harmful Algae,2004,3:331-342.
    [32] Carder K L,Steward R G,Harvey G R,et al.Marine humic and fulvic acids:Their effects on remote sensing of ocean chlorophyll[J].Limnol Oceanogr,1989,34:68-81.
    [33] Yacobi Y Z,Alberts J J,Takács M,et al.Absorption spectroscopy of colored dissolved organic carbon in Georgia(USA) rivers:the impact of molecular size distribution[J].Journal of Limnology,2003,62:41-46.
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出版历程
  • 收稿日期:  2006-02-12
  • 修回日期:  2006-07-17
  • 刊出日期:  2007-05-24

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